The syntheses of amphiphilic antimony(V)-phthalocyanines and spectral investigation on their aggregation behaviors in aqueous and non-aqueous solutions

Hiroaki Isago*, Yutaka Kagaya, Youichi Oyama, Harumi Fujita, Tamotsu Sugimori

*この論文の責任著者

研究成果: ジャーナルへの寄稿学術論文査読

13 被引用数 (Scopus)

抄録

Three amphiphilic antimony(V)-phthalocyanines have been synthesized by treating [Sb(R 4Pc)(OH) 2] + salts in concentrated H 2SO 4 and isolated as zwitter ions, [Sb(R 4Pc)(SO 4H)(SO 4)], where R 4Pc denotes tetra-substituted phthalocyaninate; R 4Pc = pc (R = H), tbpc (R = tBu), and tObpc (R = O nBu). Their solubility (R = tbpc > pc ≫ tObpc in H 2O (much improved by the presence of surfactant or alcohol) while tbpc > tObpc ≫ pc in CH 2Cl 2) and aggregation behaviors are highly sensitive to the nature of the peripheral substituents. The pc and tbpc derivatives form well-behaved J-aggregates in aqueous media in the presence of surfactant or alcohol.

本文言語英語
ページ(範囲)91-98
ページ数8
ジャーナルJournal of Inorganic Biochemistry
111
DOI
出版ステータス出版済み - 2012/06

ASJC Scopus 主題領域

  • 生化学
  • 無機化学

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