Impacts of framework Al distribution and acidic properties of Cu-exchanged CHA-type zeolite on catalytic conversion of methane into methanol followed by lower hydrocarbons

Kengo Nakamura; Peipei Xiao; Ryota Osuga; Yong Wang; Shuhei Yasuda; Takeshi Matsumoto; Junko N. Kondo; Mizuho Yabushita; Atsushi Muramatsu; Hermann Gies; Toshiyuki Yokoi

doi:10.1039/d3cy00127j

Impacts of framework Al distribution and acidic properties of Cu-exchanged CHA-type zeolite on catalytic conversion of methane into methanol followed by lower hydrocarbons

Kengo Nakamura, Peipei Xiao, Ryota Osuga, Yong Wang, Shuhei Yasuda, Takeshi Matsumoto, Junko N. Kondo, Mizuho Yabushita, Atsushi Muramatsu, Hermann Gies, Toshiyuki Yokoi^*

^*この論文の責任著者

工学科　応用化学コース

研究成果: ジャーナルへの寄稿 › 学術論文 › 査読

13 被引用数 (Scopus)

抄録

This work highlighted the significance of the Al distribution in the CHA-type zeolite in the formation of active Cu species for oxidative conversion of CH₄; isolated Al atoms in the zeolite framework are found to be advantageous for producing CH₃OH. The acid sites also played an important role in the production of hydrocarbons; produced CH₃OH is converted into hydrocarbons over the acid sites.

本文言語	英語
ページ（範囲）	2648-2651
ページ数	4
ジャーナル	Catalysis Science and Technology
巻	13
号	9
DOI	https://doi.org/10.1039/d3cy00127j
出版ステータス	出版済み - 2023/03/14

ASJC Scopus 主題領域

触媒

文献へのアクセス

10.1039/d3cy00127j

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「Impacts of framework Al distribution and acidic properties of Cu-exchanged CHA-type zeolite on catalytic conversion of methane into methanol followed by lower hydrocarbons」の研究トピックを掘り下げます。これらがまとまってユニークなフィンガープリントを構成します。

引用スタイル

Nakamura, K., Xiao, P., Osuga, R., Wang, Y., Yasuda, S., Matsumoto, T., Kondo, J. N., Yabushita, M., Muramatsu, A., Gies, H., & Yokoi, T. (2023). Impacts of framework Al distribution and acidic properties of Cu-exchanged CHA-type zeolite on catalytic conversion of methane into methanol followed by lower hydrocarbons. Catalysis Science and Technology, 13(9), 2648-2651. https://doi.org/10.1039/d3cy00127j

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title = "Impacts of framework Al distribution and acidic properties of Cu-exchanged CHA-type zeolite on catalytic conversion of methane into methanol followed by lower hydrocarbons",

abstract = "This work highlighted the significance of the Al distribution in the CHA-type zeolite in the formation of active Cu species for oxidative conversion of CH4; isolated Al atoms in the zeolite framework are found to be advantageous for producing CH3OH. The acid sites also played an important role in the production of hydrocarbons; produced CH3OH is converted into hydrocarbons over the acid sites.",

author = "Kengo Nakamura and Peipei Xiao and Ryota Osuga and Yong Wang and Shuhei Yasuda and Takeshi Matsumoto and Kondo, {Junko N.} and Mizuho Yabushita and Atsushi Muramatsu and Hermann Gies and Toshiyuki Yokoi",

note = "Publisher Copyright: {\textcopyright} 2023 The Royal Society of Chemistry.",

year = "2023",

month = mar,

day = "14",

doi = "10.1039/d3cy00127j",

language = "英語",

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Nakamura, K, Xiao, P, Osuga, R, Wang, Y, Yasuda, S, Matsumoto, T, Kondo, JN, Yabushita, M, Muramatsu, A, Gies, H & Yokoi, T 2023, 'Impacts of framework Al distribution and acidic properties of Cu-exchanged CHA-type zeolite on catalytic conversion of methane into methanol followed by lower hydrocarbons', Catalysis Science and Technology, vol. 13, no. 9, pp. 2648-2651. https://doi.org/10.1039/d3cy00127j

Impacts of framework Al distribution and acidic properties of Cu-exchanged CHA-type zeolite on catalytic conversion of methane into methanol followed by lower hydrocarbons. / Nakamura, Kengo; Xiao, Peipei; Osuga, Ryota その他.
In: Catalysis Science and Technology, Vol. 13, No. 9, 14.03.2023, p. 2648-2651.

研究成果: ジャーナルへの寄稿 › 学術論文 › 査読

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AU - Xiao, Peipei

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AU - Yasuda, Shuhei

AU - Matsumoto, Takeshi

AU - Kondo, Junko N.

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AU - Muramatsu, Atsushi

AU - Gies, Hermann

AU - Yokoi, Toshiyuki

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