4σ-1 inner valence photoionization dynamics of NO derived from photoelectron-photoion angular correlations

O. Geßner; Y. Hikosaka; B. Zimmermann; A. Hempelmann; R. R. Lucchese; J. H.D. Eland; P. M. Guyon; U. Becker

4σ^-1 inner valence photoionization dynamics of NO derived from photoelectron-photoion angular correlations

O. Geßner^*, Y. Hikosaka, B. Zimmermann, A. Hempelmann, R. R. Lucchese, J. H.D. Eland, P. M. Guyon, U. Becker

^*Corresponding author for this work

Faculty of Liberal Arts and Sciences

Research output: Contribution to journal › Article › peer-review

73 Scopus citations

Abstract

The molecule frame angular distributions of photoelectrons and photoions emitted after the 4σ^-1 photoionization of nitrous oxide molecules in the gas phase were measured. Linearly and circularly polarized light were used at a photon energy of 40.8 eV to derive a unique set of dipole transition moments and phase differences. Measured data and the derived dipole transition parameters were compared to multichannel Schwinger configuration interaction calculations. Comparisons of Schwinger configuration interaction calculations showed the capability of this method to predict the angular distributions due to correct identification of main components of the photoelectron wave expansion and their relative phase shifts.

Original language	English
Article number	193002
Pages (from-to)	1930021-1930024
Number of pages	4
Journal	Physical Review Letters
Volume	88
Issue number	19
State	Published - 2002/05/13

ASJC Scopus subject areas

General Physics and Astronomy

Cite this

@article{1b62cc24029c47ca97c2a689d771082b,

title = "4σ-1 inner valence photoionization dynamics of NO derived from photoelectron-photoion angular correlations",

abstract = "The molecule frame angular distributions of photoelectrons and photoions emitted after the 4σ-1 photoionization of nitrous oxide molecules in the gas phase were measured. Linearly and circularly polarized light were used at a photon energy of 40.8 eV to derive a unique set of dipole transition moments and phase differences. Measured data and the derived dipole transition parameters were compared to multichannel Schwinger configuration interaction calculations. Comparisons of Schwinger configuration interaction calculations showed the capability of this method to predict the angular distributions due to correct identification of main components of the photoelectron wave expansion and their relative phase shifts.",

author = "O. Ge{\ss}ner and Y. Hikosaka and B. Zimmermann and A. Hempelmann and Lucchese, {R. R.} and Eland, {J. H.D.} and Guyon, {P. M.} and U. Becker",

year = "2002",

month = may,

day = "13",

language = "英語",

volume = "88",

pages = "1930021--1930024",

journal = "Physical Review Letters",

issn = "0031-9007",

publisher = "American Physical Society",

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TY - JOUR

T1 - 4σ-1 inner valence photoionization dynamics of NO derived from photoelectron-photoion angular correlations

AU - Geßner, O.

AU - Hikosaka, Y.

AU - Zimmermann, B.

AU - Hempelmann, A.

AU - Lucchese, R. R.

AU - Eland, J. H.D.

AU - Guyon, P. M.

AU - Becker, U.

PY - 2002/5/13

Y1 - 2002/5/13

N2 - The molecule frame angular distributions of photoelectrons and photoions emitted after the 4σ-1 photoionization of nitrous oxide molecules in the gas phase were measured. Linearly and circularly polarized light were used at a photon energy of 40.8 eV to derive a unique set of dipole transition moments and phase differences. Measured data and the derived dipole transition parameters were compared to multichannel Schwinger configuration interaction calculations. Comparisons of Schwinger configuration interaction calculations showed the capability of this method to predict the angular distributions due to correct identification of main components of the photoelectron wave expansion and their relative phase shifts.

AB - The molecule frame angular distributions of photoelectrons and photoions emitted after the 4σ-1 photoionization of nitrous oxide molecules in the gas phase were measured. Linearly and circularly polarized light were used at a photon energy of 40.8 eV to derive a unique set of dipole transition moments and phase differences. Measured data and the derived dipole transition parameters were compared to multichannel Schwinger configuration interaction calculations. Comparisons of Schwinger configuration interaction calculations showed the capability of this method to predict the angular distributions due to correct identification of main components of the photoelectron wave expansion and their relative phase shifts.

UR - http://www.scopus.com/inward/record.url?scp=0037071260&partnerID=8YFLogxK

M3 - 学術論文

AN - SCOPUS:0037071260

SN - 0031-9007

VL - 88

SP - 1930021

EP - 1930024

JO - Physical Review Letters

JF - Physical Review Letters

IS - 19

M1 - 193002

ER -

4σ-1 inner valence photoionization dynamics of NO derived from photoelectron-photoion angular correlations

Abstract

ASJC Scopus subject areas

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4σ^-1 inner valence photoionization dynamics of NO derived from photoelectron-photoion angular correlations